N2
てならない
Very, Extremely, Can't help but do
昨日は徹夜して勉強してたから、眠くてならない。
I was up all night studying yesterday, so I'm extremely sleepy.
Explanation
「てならない」 means 'I can't help feeling...'. A feeling, hunch or worry is not forced; it wells up from inside and cannot be held back. It mainly follows words like 「思われる」, 「思い出される」, 「気がする」, and 「心配だ」, 「残念だ」, 「不安だ」, 「悔やまれる」. Example: 「彼のことが心配でならない」 (I can't stop worrying about him). It is a rather formal, written form.
Mixed up with
「てならない」: fits best with 「思える」, 「気がする」, 「気になる」; thoughts that arise on their own; a written register.
「てたまらない」: the usual choice for bodily sensations (pain, itching, heat, hunger, thirst) and urgent wants (〜たくてたまらない); 「てならない」 can also take them but sounds stiffer.
「てしょうがない」: you can do nothing about the situation.